Dual-frequency-comb UV spectroscopy with one million resolved comb lines
Andrey Muraviev, Dmitrii Konnov, Sergey Vasilyev, and Konstantin L. Vodopyanov
Abstract
We present high-resolution dual-comb spectroscopy across two broad UV spectral regions spanning 372–410 nm and 325–342 nm. This is achieved by generating sixth and seventh harmonics, respectively, from a low-noise 2.35 µm Cr:ZnS dual-comb laser system. The sixth harmonic band contains approximately 1,000,000 spectrally resolved comb lines, while the seventh harmonic band—around 550,000 comb lines. With the line spacing of 80 MHz, this corresponds to a resolving power of up to 10 million, offering remarkable spectral resolution.
Yudi Wu, Qiang Fu, Sijing Liang, Francesco Poletti, David J. Richardson, and Lin Xu
Abstract
We report a high-energy, picosecond, mid-infrared (MIR) optical parametric oscillator (OPO), in which a length of hollow-core-fiber (HCF) is employed to enable operation at 1-MHz repetition rate in a compact cavity format. The OPO is synchronously pumped by an ytterbium-doped-fiber (YDF) master-oscillator-power-amplifier (MOPA) system, seeded by a 1040-nm gain-switched laser diode (GSLD). Using periodically poled lithium niobate (PPLN) as the nonlinear crystal, the OPO generates signal and idler beams with tunable wavelengths in the range of 1329–1641 nm and 2841–4790 nm, respectively. The OPO provides 137-ps pulses with a maximum signal energy of 10.05 µJ at 1600 nm and a maximum idler energy of 5.13 µJ at 2967 nm. This, to the best of our knowledge, represents the highest energy MIR pulses, as well as the highest total converted pulse energy (15.18 µJ), ever achieved from a fiber laser pumped picosecond OPO.
Yudi Wu, Sijing Liang, Qiang Fu, Thomas D. Bradley, Francesco Poletti, David J. Richardson, and Lin Xu
Abstract
A compact, mid-infrared (MIR), synchronously pumped, fiber-feedback optical parametric oscillator (OPO) based on periodically poled lithium niobate (PPLN) is developed with tunable signal and idler wavelength ranges of 1472.0–1758.2 nm and 2559.1–3562.7 nm, respectively. A solid-core SMF-28 fiber and a hollow-core fiber (HCF) were used as the feedback fibers in order to compare the effect of their substantially different levels of nonlinearity. The OPO generates 1-MHz, 120-ps, MIR pulses with up to 1.50-µJ pulse energy and 11.7-kW peak power.
Demonstration of an 8-Gbit/s quadrature-phase-shift-keying coherent underwater wireless optical communication link using coherent heterodyne detection under scattering conditions
Yuxiang Duan, Huibin Zhou, Zile Jiang, Muralekrishnan Ramakrishnan, Xinzhou Su, Wing Ko, Yue Zuo, Hongkun Lian, Ruoyu Zeng, Yingning Wang, Zixun Zhao, Moshe Tur, and Alan E. Willner
Abstract
In this paper, we experimentally demonstrate an 8-Gbit/s quadrature-phase-shift-keying (QPSK) coherent underwater wireless optical communication (UWOC) link under scattering conditions at 532 nm. At the transmitter, we generate the 532-nm QPSK signal using second-harmonic generation (SHG), where the 1064-nm signal modulated with four phase levels of an 8-phase-shift-keying (8-PSK) format is phase doubled to produce the 532-nm QPSK signal. To enhance the receiver sensitivity, we utilize a local oscillator (LO) at the receiver from an independent laser source. The received QPSK data beam is mixed with the independent LO for coherent heterodyne detection. Results show that the bit error rates (BERs) of the received QPSK signal can reach below the 7% forward error correction (FEC) limit under turbid water with attenuation lengths (γL) up to 7.4 and 6.1 for 2- and 8-Gbit/s QPSK, respectively. The corresponding receiver sensitivities are −34.0 and −28.4 dBm for 2- and 8-Gbit/s QPSK, respectively.
TECHNICAL GUIDE: Covesion SFG Crystals for Laser Cooling and Trapping
Covesion’s range of MSFG crystals are most commonly used in quantum optics systems where narrow linewidth lasers are needed to access specific atomic transitions in order to manipulate and cool atoms and ions. Cooling lasers with Watt level powers are readily achievable by using high power fiber pump lasers for sum frequency generation in MgO:PPLN.
For example, the MSFG626 can be used for cooling Beryllium ions from two pump lasers at 1051nm and 1550nm which are then combined in the MSFG626, generating 626nm. This output is can then be frequency doubled to a 9Be+ ion transition at 313nm using a BBO crystal[1,2]. Similarly, our MSHG637 has been used to demonstrate cooling of Caesium atoms from 1560nm and 1077nm to 637nm, which is then frequency doubled to an atomic transition[3]. Our full range of MSFG crystals is shown below.
Part#
Pumps (nm)
Output (nm)
Grating periods (μm)
Lengths (mm)
MSFG578
1030nm + 1280-1365nm
570-587nm
8.70, 8.80, 8.90, 9.00, 9.10
1, 3, 10, 20, 40
MSFG612
1550nm + 1000-1025nm
608-617nm
10.40, 10.55, 10.70, 10.85, 11.00
1, 3, 10, 20, 40
MSFG626
1051nm + 1550-1560nm
618-628nm
11.12, 11.17, 11.22
1, 3, 10, 20, 40
MSFG637
1070nm + 1520-1590nm
628-640nm
11.60, 11.65, 11.70, 11.75, 11.80
1, 3, 10, 20, 40
MSFG647
1550nm + 1085-1160nm
638-663nm
12.10, 12.30, 12.50, 12.70, 12.90
1, 3, 10, 20, 40
To achieve efficient SFG, you ideally want the two pump beams to be confocally focussed into the PPLN (i.e. ratio of the crystal length to the confocal parameter is 1) and for both beams to be roughly equal in power. Note that for high power beams, a looser focus is recommended, avoiding back-conversion or crystal damage.
For generation of 626nm light from 1051nm and 1551nm, efficiencies of 3.5-2.5%/Wcm have been achieved[1,2]. Here, the efficiency η, is defined by
Where P is the power at each wavelength, and l is the crystal length. Lo et al. demonstrated an efficiency of 44% for the generation of 7.2W of 626nm light from 1051nm (8.5W) and 1551nm (8.3W)[1]. Here they used a 40mm long, 0.5mm thick crystal at 180C with a 58μm spot size (1/e2 radius). Further examples and technical details are summarised in the table below of some selected publications.
TECHNICAL GUIDE: Frequency Doubling Femtosecond Fiber Lasers
One of the most common applications of our crystals is for the generation of femtosecond pulses at around 780nm which can also be used as a low cost and compact alternative to the Ti:Sapphire laser.
This is typically achieved by frequency doubling a high power 1560nm Er 3+ fiber source using a 1mm long MgO:PPLN crystal (MSHG1550-0.5-xx) at room temperature (no PPLN crystal oven needed). Such a source can be used in microscopy systems for live-cell imaging, or terahertz time-domain spectroscopy where chemical fingerprints can be identified for homeland security applications.
The crystal length is an important factor when choosing a crystal for femtosecond laser frequency doubling due to the acceptance bandwidth of the device. The crystal needs to be long enough to achieve good temporal overlap of the pulses, and yet short enough to accommodate the bandwidth. The MSHG1550-0.5-xx is available in lengths as short as 0.3mm for <30-100 fs, but typically for 100-200fs pulse durations, a 1mm long crystal is recommended.
For frequency doubling femtosecond laser pulses, if the pump bandwidth is significantly wider than the acceptance bandwidth, it is still possible to achieve high conversion efficiency. The pump frequencies outside of the acceptance bandwidth can still contribute to the conversion efficiency via sum frequency generation, essentially squeezing the broadband pump into a relatively narrower-band SHG pulse [1].
Using a 1mm crystal length and 5-10μm focussed spot sizes (1/e2 radius), customers have reported efficiencies of 40-60% for ~100fs, 100MHz and 100-200mW average powers. Due to the very wide temperature acceptance bandwidth, <1mm long crystals can be used at room temperature, and with no temperature controller, for SHG at 1550 or 1560nm.
Huang et al. have reported a Multiphoton Microscopy System based on MgO:PPLN with an SHG conversion efficiency of 40% under the following conditions [4]:
The table below shows the available lengths for the MSHG1550-0.5-xx and the recommended lengths based on input pulse duration and pump acceptance bandwidth. The temperature acceptance bandwidth of the crystal length indicates that crystal lengths less than 1mm do not need to be temperature stabilised in a PPLN crystal oven. The maximum SHG bandwidth is the maximum bandwidth expected from the crystal due to its length.
Length (mm)
Pump acceptance bandwidth (nm)
Temperature acceptance bandwidth (C)
Maximum SHG bandwidth (nm)
Input pulse duration
0.3
40
265
20
<30 – 100 fs[2]
0.5
24
170
12
50 – 100 fs
1
12
90
6.0
100 – 200 fs
3
4.0
30
2.0
200 – 500 fs
5
2.4
20
1.2
0.5 – 2 ps
10
1.2
10
0.6
1 – 3 ps[3]
References
K. Moutzouris et al., Optics letters, vol. 31, no. 8, pp. 1148–50, (2006)
C. W. Freudiger et al., Nature Photonics 8, 153–159 (2014)
C. Peuntinger et al., Phys. Rev. Lett. 113, 060502
L. Huang et al., Biomed. Opt. Express, vol. 7, no. 5, p. 1948, (2016)
TECHNICAL GUIDE: High Power 780 nm for Laser Cooling and Manipulation of Rb Atoms
The manipulation of Rb atoms is commonly performed using diode-based laser systems typically producing several hundred mW of usable 780nm power. Many atom optics applications however favour higher laser power whilst maintaining a narrow linewidth and high spatial beam quality. One method is to frequency-double 1560nm fiber lasers that can deliver tens of Watts in optical power.
Covesion MgO:PPLN crystals have been used to generate as much as 11W at 780nm in a frequency-doubled 1560nm CW SHG system [1]. Furthermore, a peak power of 43W at 780nm has been achieved in a quasi-CW using two cascading MgO:PPLN crystals, with an efficiency of 66% [2]. Details about the experimental setup, SHG crystals and focussing conditions leading to these results, are discussed below.
These MgO:PPLN based laser systems have been used in several applications including, a demonstration of a quantum superposition over 54 centimetres [3], a precision gravimeter [4], a dual-species atom interferometer for BECs [5], and a new type of sensor which simultaneously measures gravity and magnetic field gradients to a high precision [6].
11W at 780nm with a single pass SHG system ANU’s Quantum Sensors and Atom laser Group demonstrated an 11.4W narrow linewidth laser source [1]. Using a 30W 1560nm fiber laser in a single-pass frequency doubling scheme, Sané et al. achieved a 6kHz linewidth 780nm laser with 36% efficiency. This corresponds to an efficiency of 0.3%/Wcm (in a low gain system, you can typically achieve 0.6%/W/cm), and the maximum input intensity to the crystal is 500kW/cm2. The system was run for over 2200hrs of operation with no reduction in power. The SHG output power is shown in Fig. 1, with an inset showing the spatial mode of the 780nm light. The 780nm source is measured to have a linewidth of 6 kHz integrated over 100ms.
Figure 1: Measured SHG output power from MSHG1550-1.0-40
The optical setup of the laser system is shown in Fig. 2, with the 30W 1560nm laser, MgO:PPLN crystal, and Rb cell for locking the seed laser. A standard MSHG1550-1.0-40 was used as the SHG crystal, heated in a PV40 oven with an OC1 temperature controller. The crystal parameters and focussing conditions used were:
Period = 19.5µm, T = 81.60C
Crystal length = 40mm, Thickness = 1mm
1/e2 diameter to a 50 mm focal length lens = of 1.1 mm
equivalent to calculated 45µm spot size ( 1/e² radius) in the centre of the crystal length
maximum input intensity to the crystal = 500kW/cm²
Figure 2: Experimental setup of the 11W SHG laser system
The Kasevich group at Stanford University have demonstrated 43W of quasi-CW 780nm light [2]. Chiow et al. describe a cascaded single pass SHG system using two MgO:PPLN crystals. The system is pumped with two combined 1560nm 30W fiber amplifiers, and by adjusting the relative phase between these two sources, the temporal profile of the 780nm output can be controlled. With a combined pump power of 65W, a peak power of 43W is achieved at 780nm, corresponding to an efficiency of 66%. With a single crystal, an of 52% efficiency is achieved. The SHG output peak power from an single crystal and from two cascaded crystals is shown in Fig. 3. The data from Sané et al. are also shown in green, showing almost identical results.
Figure 3: Measured output power from cascaded MSHG1550-1.0-40 crystals (red). Data from Sané et al. is also shown in green.
The optical setup of the laser system is shown in Fig. 4 with the two fiber amplifiers (FA) and two cascaded MgO:PPLN crystals. Standard MSHG1550-1.0-40 crystals in PV40 ovens were used, from which a period of 19.2µm was selected, at an operating temperature of 150C. The pump was focussed into PPLN1 with a 50mm focal length lens, a curved mirror (CM) with ROC 10cm collimated the output beams which were then focussed into PPLN2 with another CM. Analysis of the 780nm spatial beam profile from the cascaded system measured a beam quality of M2= 1.15+/-0.2.
Figure 4: Experimental setup of the cascaded SHG system
References
S. S. Sané et al., “11 W narrow linewidth laser source at 780 nm for laser cooling and manipulation of Rubidium.,” Opt. Express, vol. 20, no. 8, pp. 8915–9, 2012.
S. Chiow et al., “Generation of 43 W of quasi-continuous 780 nm laser light via high-efficiency, single-pass frequency doubling in periodically poled lithium niobate crystals.,” Opt. Lett., vol. 37, no. 18, pp. 3861–3, 2012.
T. Kovachy et al., “Quantum superposition at the half-metre scale,” Nature, vol. 528, no. 7583, pp. 530–533, 2015.
P. A. Altin et al., “Precision atomic gravimeter based on Bragg diffraction,” New J. Phys., vol. 15, no. 2, p. 23009, 2013.
C. C. N. Kuhn et al., “A Bose-condensed, simultaneous dual-species Mach–Zehnder atom interferometer,” New J. Phys., vol. 16, no. 7, p. 73035, 2014.
K. S. Hardman et al., “Simultaneous Precision Gravimetry and Magnetic Gradiometry with a Bose-Einstein Condensate: A High Precision, Quantum Sensor,” Phys. Rev. Lett., vol. 117, no. 13, p. 138501, 2016
Photon Pair Source based on PPLN-Waveguides for Entangled Two-Photon Absorption
Tobias Bernd Gäbler, Patrick Hendra, Nitish Jain, Markus Gräfe
Abstract
Fluorescence excitation by absorption of entangled photon pairs offers benefits compared to classical imaging techniques, such as the attainment of higher signal levels at low excitation power while simultaneously mitigating phototoxicity. However, current entangled photon pair sources are unreliable for fluorescence detection. In order to address this limitation, there is a need for ultra-bright entangled photon pair sources. Among the potential solutions, sources utilizing nonlinear waveguides emerge as promising candidates to facilitate fluorescence excitation through entangled photons. In this paper, a source consisting of a periodically poled lithium niobate waveguide is developed and its key characteristics are analyzed. To demonstrate its suitability as key component for imaging experiments, the entangled two-photon absorption behavior of Cadmium Selenide Zinc Sulfide quantum dot solutions is experimentally investigated.
Recent Progress in Short and Mid-Infrared Single-Photon Generation: A Review
Arianna Elefante, Stefano Dello Russo, Fabrizio Sgobba, Luigi Santamaria Amato, Deborah Katia Pallotti, Daniele Dequal and Mario Siciliani de Cumis
Abstract
The generation of single photons in the mid-infrared spectral region is attracting the interest of scientific and technological research, motivated by the potential improvements that many important and emerging applications, such as quantum sensing, metrology and communication, could benefit from. This review reports the progress in short and mid-infrared single photon generation, focusing on probabilistic sources based on the two non-linear processes of spontaneous parametric downconversion (SPDC) and four wave mixing (FWM). On one hand, numerical simulations of mid-infrared SPDC are described as a powerful tool to assist and guide the experimental realization, along with the implementation and engineering of novel non-linear materials. On the other hand, the advantages offered by FWM in silicon waveguides in terms of integration, miniaturization and manufacturability are presented, providing an optimal technology for integrated quantum applications.
Quantum and non-local effects offer over 40 dB noise resilience advantage towards quantum lidar
Phillip S. Blakey, Han Liu, Georgios Papangelakis, Yutian Zhang, Zacharie M. Léger, Meng Lon Iu & Amr S. Helmy.
Abstract
Non-local effects have the potential to radically move forward quantum enhanced imaging to provide an advantage over classical imaging not only in laboratory environments but practical implementation. In this work, we demonstrate a 43dB higher signal-to-noise ratio (SNR) using a quantum enhanced LiDAR based on time-frequency entanglement compared with a classical phase-insensitive quantum imaging system. Our system can tolerate more than 3 orders of magnitude higher noise than classical single-photon counting quantum imaging systems before detector saturation with a detector dead time of 25ns. To achieve these advantages, we use non-local cancellation of dispersion to take advantage of the strong temporal correlations in photon pairs in spite of the orders of magnitude larger detector temporal uncertainty. We go on to incorporate this scheme with purpose-built scanning collection optics to image non-reflecting targets in an environment with noise.